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/Keywords (nanowire; optical properties; heterostructure; near infrared emission)
/Title (Near-infrared emission from spatially indirect excitons in type {II} {ZnTe/CdSe/\(Zn,Mg\)Te} core/double-shell nanowires)
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/Subject (ZnTe/CdSe/\(Zn,Mg\)Te core/double-shell nanowires are grown by molecular beam epitaxy by employing the vapor-liquid-solid growth mechanism assisted with gold catalysts. A photoluminescence study of these structures reveals the presence of an optical emission in the near infrared. We assign this emission to the spatially indirect exciton recombination at the ZnTe/CdSe type II interface. This conclusion is confirmed by the observation of a significant blue-shift of the emission energy with an increasing excitation fluence induced by the electron-hole separation at the interface. Cathodoluminescence measurements reveal that the optical emission in the near infrared originates from nanowires and not from two dimensional residual deposits between them. Moreover, it is demonstrated that the emission energy in the near infrared depends on the average CdSe shell thickness and the average Mg concentration within the \(Zn,Mg\)Te shell. The main mechanism responsible for these changes is associated with the strain induced by the \(Zn,Mg\)Te shell in the entire core/shell nanowire heterostructure.)
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ZnTe/CdSe/(Zn,Mg)Te core/double-shell nanowires are grown by molecular beam epitaxy by employing the vapor-liquid-solid growth mechanism assisted with gold catalysts. A photoluminescence study of these structures reveals the presence of an optical emission in the near infrared. We assign this emission to the spatially indirect exciton recombination at the ZnTe/CdSe type II interface. This conclusion is confirmed by the observation of a significant blue-shift of the emission energy with an increasing excitation fluence induced by the electron-hole separation at the interface. Cathodoluminescence measurements reveal that the optical emission in the near infrared originates from nanowires and not from two dimensional residual deposits between them. Moreover, it is demonstrated that the emission energy in the near infrared depends on the average CdSe shell thickness and the average Mg concentration within the (Zn,Mg)Te shell. The main mechanism responsible for these changes is associated with the strain induced by the (Zn,Mg)Te shell in the entire core/shell nanowire heterostructure.
bibtex/arxiv/2109.00272
bibtex/citationkey/Wojnar_nt_2021
bibtex/file/:myArticles/Wojnar_nt_2021_accepted.pdf:PDF
bibtex/journal/Nanotechnology
bibtex/month/September
bibtex/note/7 pages
bibtex/number/49
bibtex/pages/495202
bibtex/volume/32
Piotr Wojnar
Jakub Krzysztof Płachta
Anna Reszka
Jonas Lähnemann
Anna Kaleta
Slawomir Kret
Piotr Baranowski
Maciej Wójcik
Bogdan J. Kowalski
Lech Tomasz Baczewski
10.1088/1361-6528/ac218c
Near-infrared emission from spatially indirect excitons in type {II} {ZnTe/CdSe/(Zn,Mg)Te} core/double-shell nanowires
2021-09
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